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Climate change bio

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atmosphere (waaay back)
Originally similar to sun
⬢ Dominated by
o Hydrogen and helium
o Small amounts of methane, water vapor, ammonia, CO2, and gaseous nitrogen
Slowly things began to change
⬢ Hydrogen and helium disappear (small molecule mass)
⬢ Short wave UV radiation began to decompose H2O and NH3
o Resulted in more O2 and N2








Volcanoes become a factor

⬢ Eruptions release
o CO2
o Water vapor
o N2
o Sulfur
o Volcanic ash







ozone develops, and O becomes available
Ozone layer developed
⬢ O3 layer developed as the stratosphere formed
⬢ Provided a shield from harmful UV radiation and allowed life forms to develop
Photosynthesis arrives as O2 becomes more abundant
⬢ The evolution of photosynthesizing organisms became possible
o Cyanobacteria
o Algae
o Plants








then comes humans
⬢ Human activities
o Discovery of fire for heating and cooking
o Development of villages and towns
o Development of organized agriculture
o Population growth
o Habitat destruction
o Pollution
⬢ Industrial revolution
o In 300 years there have been increases in
⬢ CO2 and H2O vapor
⬢ Methane
⬢ Sulfur and Nitrogen
⬢ Ozone (photochemical oxidant cycle)
⬢ Synthetic chemicals














Troposphere

o 8-12 km up from the earths surface
o temperature decreases with height
o unstable turbulence, thermal energy
o weather is found here, occurs when cold and warm fronts interact





stratosphere
o 12-48 km
o contains the ozone layer
⬢ relatively stable region
⬢ few clouds, horizontal ⬦?
⬢ Temperature increases with height





Assessing the Effects of Air Pollutants

Plants and Air Pollutants


⬢ Most more responsive than humans at lower concentrations
⬢ Easier to work with, large numbers can be used
⬢ Better data bases are available for dose/response than for humans




Assessing the Effects of Air Pollutants

Pollutant uptake by plants

⬢Via stomata
o Gases taken up during gas exchange in photosynthesis
⬢Via cuticle
o Wet and dry deposition of gases, ions and particles
⬢Via soil
o Uptake by xylem from soil






Assessing the Effects of Air Pollutants

Plant Responses

⬢Acute injury
o Necrosis, visible
o Usually means high exposure/short time
⬢Chronic injury
o Chlorosis, pigmentation
o Usually means low levels/long time
⬢Growth responses
o Measurable effects on growth/reproduction
o Combination of acute/chronic









Assessing the Effects of Air Pollutants

Effects Detection Approaches

⬢Reductionist
o Full control, not natural, dose/response
⬢Semi-reductionist
o Less control, more natural, dose/response
⬢Natural conditions
o Ambient, little control, natural, no dose/response






Assessing the Effects of Air Pollutants

Effects Detection Approaches (more in depth)

Reductionist Approach
⬢ Grow plants under controlled conditions
Semi-reductionist
⬢ Chambers of various types
⬢ Open air fumigation systems
Natural Exposure
⬢ bioindicators
⬢ Fields plots
⬢ Potted plants in a the field
⬢ Concentration gradients
⬢ Tolerant vs. sensitive plants
⬢ Antioxidant chemicals












Assessing the Effects of Air Pollutants

Bioindicators and biomonitors

⬢Bioindicators
o Qualitative assessment
o Something has happened
⬢Biomonitors
o Quantitative assessment
o Dose/response approximated






Assessing the Effects of Air Pollutants

Types of Bioindicators and Biomonitors

⬢Sentinels
o Known sensitive organisms introduced into an area
⬢Early warning: local monitoring abatement
⬢Require special care
o Tobacco plants are bioindicators
⬢Detectors
o Naturally occurring species that may show a response
⬢Ecologically significant
⬢Locally important
o Indigenous plants
⬢ Exploiters
o Presence indicates disturbance and or pollution
⬢Abundance indicates due to lack of competition
o Stinging nettles
⬢Accumulators
o Take up and accumulate chemicals
⬢Can be measure
⬢Quantitative
o Lichens
⬢Bioassays
o Plants used for lab assays
⬢ Biochemical analyses
⬢ Physiological responses























Environmental Molecular Epidemiology

Biomarkers

⬢ Molecular biomarkers
⬢ Tools of molecular analysis
⬢ Changes in DNA
⬢ Leading to
o Susceptibility
o Exposure
o Early disease incidence







Environmental Molecular Epidemiology

Promise of Biomarkers

⬢ Early detections of disease
o Catch it while it is still reversible
o Before the damages are permanent
⬢ Custom-managed treatment
⬢ Difficult to identify with other confounding variables





Environmental Molecular Epidemiology

PAHs

⬢ Polycyclic aromatic hydrocarbons
⬢ Incomplete combustion
o Coal Fossil fuels
o Cigarettes
⬢ Widespread





Environmental Molecular Epidemiology

Epigenetics

⬢ A different kind of biomarker
⬢ Heritable environmentally induced
o The environment almost activates these genes, so its induced but inherited
⬢ Changes in gene function
⬢ Mutations in DNA code letters
⬢ PAHs appear to be involved
⬢ Different than DNA adducts







Environmental Molecular Epidemiology

DNA Methylation


• Attachment of methyl groups to DNA
• “silences” genes
• prevents protein synthesis
• decreases disease suppression





Nitrogen


Constructing the Nitrogen Cycle
⬢ Under Natural Conditions





⬢ Aerial sources
o Fixation of N2 from air
o Inorganic N from rain, lightning, volcanoes
o Ammonia from air

⬢ Uptake by plants and soil

⬢ Wind blown aerosols with N forms

⬢ Terrestrial events
o Ammonia or nitrates taken up by plants used for amino acids
o Animal wastes, dead plants and animals broken down by bacteria and fungi to release ammonia












Human Interference disrupts the equilibrium of the Nitrogen Cycle

⬢ Human energy requirements are met by combustion
o Natural gas
o Oil
o Coal, wood, plant biomass
⬢ This releases
o CO2
o VOC
o Nitrogen compounds









Nitrogen Emissions to the Troposphere and stratosphere
⬢ Oxidized N fro fossil fuel combustion
o NO and NO2
⬢ Reduced N
o NH3
⬢ Agriculture
 Animal excrement
 Fertilizer
⬢ Wildlife
 Animal excrement









Nitric oxide NO
o Released by microbial actions on fertilizer on and in soil
o Active in the photochemical oxidant cycle
⬢ E.g. ozone formation

Global Population and the Nitrogen Cycle

⬢ Until the 20th century
o Nitrogen availability limited crop production and restricted population growth
⬢ The synthesis of ammonia and resulting abundance of nitrogen fertilizer changed all that
⬢ The availability of ammonia and fertilizers derived from it has eliminated a fundamental restriction on food production and allowed massive increases in population





Harber-Bosch Synthesis of Ammonia
Ammonia is formed when nitrogen and hydrogen are combined at high pressure and high temperatures in the presence of the catalysts osmium and uranium

Ammonia and Fertilizers
⬢ Ammonia can be used directly as a fertilizer or as ammonium nitrogen
⬢ Or used to make nitrate nitrogen fertilizers
⬢ Making fertilizers from ammonia requires electricity generated by combustion of fossil fuels



Nitrous Oxide in the Air

⬢ Bacteria in soil break down nitrates and release N2O into the air
⬢ Molecules are long lasting and act as reradiative gases
o 200 times more absorbent than CO2
⬢ N2O migrates slowly to stratosphere reacts with O3 and destroys it





sulfur Behavior in Air
⬢ Sulfate particles, SO2 and H2S
o H2S -> SO2 -> SO4 dry deposition
o S->SO2->SO3 +H2O->H2SO4 wet deposition



Sulfur Removal from Air
⬢ Sulfur is recirculated to land and sea by
o Precipitation
⬢ Wet deposition
o Particle settling
⬢ Dry deposition
⬢ Plant foliage and moist soil can also remove SO2 directly from air






Human Input of Sulfur

⬢ Combustion of fossil fuels
o Power plants
o Home heating
o Vehicles
o Manufacturing
⬢ Petroleum refining
⬢ Metal smelting
⬢ Acid drainage from mines









Sulfur Dioxide SO2

⬢ The most extensively studies air pollutant since the industrial revolution
⬢ SO2 is a point source pollutant
⬢ S is present in combusted materials and released by heat of combustion
⬢ S reacts with O2 in the air to form SO2





Dispersion Patterns of SO2

• From “short stacks”
o Graded zones of SO2
o Concentrated to dilute
o Zones called “isopleths”
o Following prevailing winds
• From “tall stacks”
o Dispersion over wide area with little contact with the ground
o Long range transport by prevailing winds
o “The solution to pollution is dilution”










Complete Combustion

⬢ At high temperatures
⬢ Fuels are rapidly oxidized to O2 yielding large amounts of heat and light
⬢ Plus products of complete combustion
o CH4 + 2O2 yields CO2 + 2H2O
o (CO2 & H2) are reradiative gases
⬢ It has a Blue flame







Incomplete Combustion

• Much of the carbon in fuels is not converted to CO2
• Some is only partially oxidized to carbon monoxide CO
• Some remains as elemental or organic carbon in particulated emitted as smoke
• Everything we have is inefficient and incomplete
o i.e. : lawn mowers, chainsaws, cars, pretty much everything except clean burning furnaces
• It’s the real cause of our problem
• It has a yellow flame








Combustion

PAHs

⬢ Compounds with two or more aromatic (benzene) tings which are fused together when a pair of carbon atoms is shared between them
⬢ Lower molecular weight compounds (2-3 ring group) are toxic

⬢ Produced at lower temperatures in wood stoves and furnaces
⬢ Higher temperatures in fireplaces destroy PAHs
⬢ Diesel engines also produce PAHs






combustion

Trucking Industry and PAHs


⬢ Very popular in the western part of the country
⬢ Little particles are emitted from the smoke stacks on trucks
o PAHs
⬢ Have begun to put trucks onto trains to reduce this, but trains still have incomplete combustion so you can never really get away from it





Combustion

Low Molecular Weight Hydrocarbons


• Formed during fuel combustion in gasoline and diesel engines
• These “unburned” hydrocarbons are even less oxidized than CO
• Become part of the photochemical oxidant cycle with anthropogenic influence
• Come out of your tail pipe. Don’t go away.





Nitrogen Compounds

⬢ High temperature combustion encourages the formation of NOx (NO + NO2)
o beginning of the cycle that produces ozone
⬢ Photochemical oxidant cycle
⬢ Acidic deposition cycle





combustion

stuff to be familiar with

Volcanoes
• Natural source of
o Sulfur
o Nitrogen
o Ash
o Toxic gases
Chlorine Compounds
• Methyl chloride – wood
• Hydrogen chloride - incineration of plastics (PVC)
Incineration of Plastics
• Incineration of plastics in furnaces results in production of carcinogenic chlorinated compounds
o PCDFs
• Dinenzofurans
o PCDDs
• Poly-chlorinated dibenzodioxins
o Dioxins
• Tetrachlorodibenzo-p-dioxin
Metals
• Found as impurities in fuels and mining ores
• Highest in coal
• Released as trace elements in ash and smoke
• Distributed by wind away from point sources






















combustion

Fire in the forest

• Surface fire
o Consumes litter and debris on the ground
o Kills herbaceous plants and woody seedlings
o Scorches the bases of large trees
• Ground fire
o Consumes organic layer under debris
o Combustion is down to the underlying mineral layer
o This prevents seedling regrowth
• Crown fire
o Canopy or “crowns” are consumed by fire
o Requires abundant debris and litter on ground and winds to bring flames to the treetops











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